PA4001 Rheology in Polymer Processing Syllabus:

PA4001 Rheology in Polymer Processing Syllabus – Anna University PG Syllabus Regulation 2021

COURSE OBJECTIVES:

 To understand the conformational property of polymer chain using different models.
 To study the chain conformation in polymer solution and melt based on thermodynamics.
 To introduce fundamental flow properties and methods used to investigate the flow behaviour under stress.
 To understand the flow behaviour in different processing methods.
 To understand the concept of melt rheology & rheometry

UNIT I MOLECULAR CONFORMATION AND CONFIGURATION

Potential and conformational energy of molecules-polymer conformation and configuration–isomerism in polymers- stereo isomerism, geometrical isomerism, sequential isomerism. Conformation of an ideal chain-mean square end to end distance-freely jointed and freely rotating chain model, worm like chain model, hindered rotation model. Radius of gyration of an ideal chain. Real chain- excluded volume, Flory theory of polymer in a solvent, deforming real and ideal chains.

UNIT II ELASTICITY

Thermo elasticity-Thermodynamics of rubbers–Flory construction- entropic and energetic contributions to the elastic force in rubbers–unentangled rubber elasticity-Affine network model- Phantom network model-entangled rubber elasticity-Edwards tube model-Mooney-Rivlin model

UNIT III SOLUTION PROPERTIES

Polymer solutions-theta condition-Thermodynamic view of miscibility-upper critical solution temperature (UCST)-lower critical solution temperature (LCST)-Concentration regimes in polymer solutions Viscoelasticity-elastic deformation-irrecoverable deformation-models of viscoelasticity-Voigtkelvin-Maxwell-Burger models-WLF equation-TTS curve-Boltzman superposition principle, stress relaxation-creep and creep recovery

UNIT IV FLOW BEHAVIOUR

Basics of rheology- shear stress-shear strain-strain rate-different types of fluids-Newtonian and Non Newtonian fluids- flow behaviour of different Non- Newtonian fluids-zero shear viscosity steady shear and oscillatory shear experiments. Methods to measure flow properties-capillary rheometer-parallel plate rheometer-cone and plate rheometer-Cup and cone viscometer. Measurement of normal stresses. Theories of viscosities of dilute and concentrated Solutions.

UNIT V MELT RHEOLOGY AND RHEOMETRY

Rheology of dilute and concentrated suspensions, Flow behaviour of polymer melts during Injection moulding-Extrusion: Film extrusion, Sheet extrusion and Blow mouldings. Bubble inflation rheometer, compression rheometer, stress relaxation instruments. Torque rheometers, rotational & sliding surface rheometers and their use in determining processability.

TOTAL: 45 PERIODS

COURSE OUTCOMES:

At the end of the course, students will be able to
CO1 Know the conformational change of polymer chains in solution and melt
CO2 Analyze the various thermoelasticity properties & thermodynamics process
CO3 Relate the polymer rheology to properties of polymeric materials and processing
CO4 Understand and measure the basic flow properties of polymers.
CO5 Apply the concept of rheology & rheometry for industrial application.

REFERENCES:

1. Elements of Physical Chemistry: S. Glasstone and D. Lewis, Macmillan India Press, Madras, 1995.
2. Crawford, Roy James, and Patrick J. Martin. Plastics Engineering. Butterworth-Heinemann, 2020.
3. Introduction to Polymer Viscoelasticity: J.J. Alkonis and W.J.Macknight–Willey Inter Science, New York, 1982.
4. Polymer Melt Rheology: F.N.Cogswell, George Goodwin Ltd. and P. R. Londo, John Wiley and Sons, 1981.
5. Polymer physics: Michael Rubinstein and R.H. Colby, Oxford University press ,2003
6. Polymer Physics: Ulf W. Gedde, Chapman & Hall, 1995
7. Rheology of Polymers: G.V.Vinogradov and A.YaMalkin, Mir Pub, Moscow, 1980.
8. Viscoelasticity of Polymers: D.D.Ferry III Edn. John Willey and Sons, New York, 1981.